Диссертация (1150357)

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«-»-02.00.11 –μ. .201522-Дқ-(Ж-қ)N-----N-. .1-(4-)3...................................................................................................................... 6I.................................................................................... 13I.Қ......................................................................................... 13I.Қ.Қ....................................................................................................................... 13I.Қ.қ........................................................................................................ 15I.Қ.3..................................................................................................................... 19I.қ.................. 21I.3............................................................................................................................

29I.3.Қ........................................................... 29I.3.қ............................................................................................................ 33I.3.3.................................... 42I.3.ζ..................................................... 45I.ζ.II.-.................................. 50......................................... 53II.Қ.......................................................... 53II.қ............................................................................. 59II.қ.Қ....................................................... 594II.қ.қ...................................................................................... 60II.қ.3.....................................................................

63II.3......................................... 64II.3.Қ......................................................... 64II.3.қ..................................................................... 68II.3.3.. ..........................................................................................................

72II.3.ζ................................................. 74III........................................................ 76σКCХ 76III.Қ.III.Қ.Қ................. 76III.Қ.қ.,................................................................................... 79III.Қ.3................................................................................................................. 80III.Қ.ζ.................................................................... 82III.Қ.η..............................................................................

87III.қ....................................................... 905III.қ.Қ.(a = 0.қ3),................. 90III.қ.қ.(a = 0.қ3) ........................................................................................................... 91III.қ.қ.Қ(a = 0.қ3) .... 91( = 0.қ3)III.қ.қ.қ................................................... 96III.қ.3.(a = 0.ηη) .........................................................................................................

100III.қ.3.Қ(a = 0.5η) .. 100( = 0.ηη)III.қ.3.қ................................................. 105III.қ.ζ.(a = Қ.0қ) ......................................................................................................... 111III.қ.ζ.Қ(a = 1.0қ) .. 111( = Қ.0қ)III.қ.ζ.қ................................................. 115III.қ.η( = 0.19) ......................................................................................................... 1206III.қ.η.Қ.( = 0.19) ...........

120( = 0.Қλ)III.қ.η.қ................................................. 122III.қ.θ( = 0.42) ......................................................................................................... 127III.қ.θ.Қ.(a = 0.42) ........... 127( = 0.ζқ)III.қ.θ.қ................................................. 131III.қ.7............................................................................ 137III.қ.κ................................................

141III.3.,........................................................................................ 153III.3.Қ.( = 0.ηη( = 0.ζқ)III.3.қ.......................................................... 153( = 0.23( = 0.Қλ)))........................................................... 154III.ζ.......... 155III.η.-..................... 1577III.η.Қ.-.......................................

157III.η.қ.-.................................................................... 159..................................................................................................................... 163........................................................................................... 1651 ........................................................................................................ 186қ ........................................................................................................

1888:,.қ0,,,,,,,(,),.,–,,,,(,,,).,,,-..,-.,9(),.,..,,.,,, «»,.,.,,(),.-,(),.,,10,-.;μ();NaCl-;,,;,-;;.:,,11,;–(V2)( / «» ( ),)(k11/b11),(W2),-(φ )-(r3 );:,.,,,,.,(,).,:((Uef),(Sm)W)0.Қλ – Қ.0қ9.0)(3.0 –,NaCl.,W;12σКCХ--(-,).-.σКCХ,;,-,.,;..;,-()( = 0.55= 0.ζқ;= 0.қ3= 0.Қλ),;-,.,,,13–..:μ.,қθ-қκ. Ққ-Қη,қ0Ққ .; III»,-«"" қ0Ққ;17(қ0Ққ .; 8-–Iμ, қҚ – қθқ0Қ3.); III«»,, қη-қθ-–қ0Қ3 ; IV Internationalconference on colloidal chemistry and physicochemical mechanics. Moscow, 30 June –05 July, 2013; 9th Saint-Petersburg Young Scientists Conference.

November 11-14,2013 Saint- Petersburg; IV«»,, Қζ-Қη-–қ0Қζ;.–Iμ Қκ-(,қ0Қζ .);, ., қҚ – қηқ0Қζ ; Vё»«6-102014; 10th Saint-Petersburg Young Scientists Conference. November 10-14, 2014 Saint- Petersburg; II«».,-Қ7«қ0Қζ ;-2015»,2015; V«, қ0-қҚ;-––»,I(-μ Қλ, қ0 – қζқ0Қη14.); IV3–«-20Қη», .қ0Қη ; III, .-қλ-–Ққ0Қη ;Modern problem of polymer Science.

11th International Saint-Petersburg Conference ofYoung Scientists. November 9-12, 2015 Saint- Petersburg; III«»., Қ0-ҚҚ-қ0Қη .:36,,Қ–,3 –,, 32,.:,(,(қҚ37Қ, Қη),қ,),,Қλ2,.:,,.–. .. . ... .. . .,; . . . . .; . . . . .,. . . . ..15I.I.1.I.1.1,,,,[1-7].().0.Қ–Қ0,η% [8-10].,,-[11].,.,().(-),,.,,[12,13].,,,–μ(II),(қ-(-қ),)–(, қ)-..16)(,..,,(),,[13-19]..()./..,,[20]...«,),,.»(.17I.1.2,.,,,,[21-23].(),,,,.–.-,,.,,,.[24,25]().,.().,,,–,.,,[26],-18.,қθ%ζ7%,.,,.,,.,,,қ0–30 %.[27]ζ,ζ’--(ζ-).,.(),,[28].,,,.,.,,,.,.19,()Дқλ,30Ж,,..Д3ҚЖ(()).,,,.,,Д3қЖ.,,«,»,,,,,,,.,.Д33Ж.,20.ηҚη,,.%.,,.,Д3ζ-35].Д3θЖT. Delair300η00,,NH2, қ·Қ0-3/ .,.λ.Д37ЖR.

Pelton-NN--(-)().,.,21.I.1.3,.(,)(,,)–Д3κ-ζ3Ж., . .,.,,,Дζζ,ζηЖ.( ,,).H. Kavaguchi [46-ζκЖ(-N.),,,,.ДζλЖT. Taniguchi-α-22.,,.,қ0ζ00 ,,,,..,(NaCl)Қζ0ζλ0/ζ0ºқ0º.,,,.. .,,.D. YuД50Ж(). M. Muller [51Ж.,(,),. D. Nagao [52Ж.θG.23.ηη0(),...,,.-,....[40,45],.I.2..,,. .().,,.().–.24.(.,)–(Қκ7λ ) –.Дη3ЖXXДηζЖ,,;.,,.ДηηЖ,,.,,,..().ДηθЖ,.,,,,.,.,,,,,.25,-,-,,,,.,,,,Дη7Ж,..,( -)–,.,,,.. .. .ДηκЖ,φd-,,. ..φd.,-.,-,,Дηλ,θ0Ж.φd.φd (26ДθҚЖ).... Д62],φd–.,,.,[63-65]φ d-,.-φd-,(),.,,,«,».,..,,.,.,.27,,.,,.,,,,.ё,Дθθ-68].,,,,«.»ДθλЖ.Д70,71]..H.Morgan [72](U )-,..U,,,,..-,U,( r>Қ0),.r<Қ0μ28κ=√–(1.6×10-19,0С� 0(1.1)�,/ , z–, e–ε–),–(κ.κη·Қ0-12 / ),(Қ.3κ×Қ0-23),.

.–k–(қλκ ).. Д73-75Ж.,.,,,,.μU ef H l  h4  t  I(1.2)Uef –,,; h–2/( · );–,; l–t, ; K –(); t –, ;I–-1 -1.,. ., .. ДθηЖ,NaCl.Қ0-2/ ,α,,29.,.A. Jódar-Reyes. Д76].ГОЭК SТгОЫ IV(εКХЯОЫЧ IЧЬЭЫЮЦОЧЭЬ).,,,.,NaClҚ0 -2/ .μ..Uef-.,r>>1-SmU ef (1.3) 0μr<<Қ Hk3 U ef 2  0(1.4)30–, ; –;12/ ),0–(κ.κη·Қ0-–· .,μ,.,-.,.(,,μ Al2O3, TiO2ZrO2) [77-81Ж,.,..Chassagne,.Ibanez [82,83Ж-KCl(MgCl2εКХЯОЫЧ ГОЭКSТгОЫ σКЧШ (ГОЭКσКЧШ),Malvern ZetaSizer 3000HSA (Zeta3000)).-(0.Қ-Қ000)/ .MgCl2.,«».,(«»)Дθ3Ж.31,,.

.«»,Д64,6ηЖ,.,J. Molina-BШХıvar [84Ж.,-–ГОЭК-Sizer IV (MalvernIЧЬЭЫЮЦОЧЭЬ),(NaCl)ζ00./ .Дκ5Ж-(зҚ00).,(3.θ3.κ).-,-..I.3I.3.1.,,.32, . ..,().. .,–Дκ6Ж.,,,. ..«»,,Дκ7].–,,,..,,.. .Д88,κλЖ(V).(h):( h)  dVdh(1.5),,.μ,,(h) =m(h)+μe(h)+a(h)+s(h)+...(1.6)33m(h)–,,e(h)–-,,a(h)–,s(h)–,,..(),..,.-.Қ-Қ00..F.London [90Ж,-Дλ1,92Ж.,. ..,.(-),Дλ3].,(,).,Дλ4Ж.34«».(Қ0),..,ДκλЖ,(. .. .).. Дλ5-99Ж,.... .. .[100-103Ж.ДҚ04].. ..ДҚ05-109Ж,,< Қη°,> ζ0°.,.-...().35,..,.,,1.3.3.I.3.2..[111,112].–--(-).μ,.,,,.,,–.«,», . ..,,.36,,..Қ.Қ.().,h.–,–=,,��=exp⁡exp⁡0̃�̃�exp⁡ − κℎ−+Қ= ℎ(1.7)̃�(1.8)�̃.z�̃c,.-..,-,37.()μ= −�/А–-�ℎ ,(1.9),,.,,.,,,h [93,140](Қ.Қ.қ.).,...Қ.қ..қ,.,.

..,Д93,140Ж.(38),.,.,...,-.,Ve, Vm,,.,().,.J. Maroto,F. de las Nieves ДҚҚ3Ж.,,, . ..ДҚҚζЖ F. de las Nieves.,ё,,«»«».39,,-«»,,,,-,.,Na+,. ... ДҚҚηЖJ. Molina-Bolívar.,.,.,..,ДҚҚθЖ,,,,,,.,.,,,. ...[117-Ққ0Ж,7θ°.,,40–,-,–COOH (S-COOH).,, . ..,S-COOH,.M. Romero-Cano ДҚқҚЖ.,,.,,,.,.,,Д122,123].ДҚқ4] S. Sauery,.,..(),қ0%ДҚқ5Ж,.41,.,,.,μ,–.,.-ДҚқ6Ж,,.,., . ..ДҚқ7].ДҚ28Ж,..,,.,.42.(),.,ДҚ29Ж,,(Қ00 < d < қ00).R.

Ottewill, J. Shaw [130Ж,. G.Wiese, T.Healy. [131Ж0.030 – 0.қҚҚ µ ,.ηҚ00.0ηµ ,,.φd30қ0.[132Ж,,.,Д133Ж≈Қ00,.κλ-κқ3.,. .,[134],.,43φ0,C (r),,φ0 =const...ДҚ34Ж,.,.ДҚ35Ж..,μ,..ДҚ36Ж,,.,.,.ДҚ37,138Ж,,,,,,..44I.3.3..ДҚ39Ж,.,,(R),( . .), . .--.nttn01/2∑∞=≡==D (1.38×10-23· ;r–),–()μ=+ � ��+(1.10),� /(1.11)��, k–(қλκ);–,, ..ДҚζ0Ж,μ�= �D–,, ΔV –(), k ––�∆���−(1.12),,,,–.45,T1/2 ()–,(nt)(n0).1/2–= � �,. .(1.13),.(Қ.Қ3)1/n-tμ=,+(1.14)� /,.,(R=2r),(Қ.Қ3),μ/(Қ.Қη)=�(1.15)�T1/2,, .

..,,.ДҚζҚ,142],.,ДҚζ3].46μҚ.(Қ.Қζ)қ.,(Қ.Қη)3.,.W(v . )(vW=v . /vҚ (W=1) [144Ж.=T1/2():)/T1/2,1.14, ,W,Қ (WҚ),«».[145-147Ж,(R2r;,Rr1+r2).,.,,(W<Қ)0.Қ(KClNaCl)/,Д148-151].–(()),().,...47.Қ.3,,()[152]..Қ.3.,.қ-3.(WҚ),ДҚ54Ж[153].,.I.3.4,,,48.,(),,,.,.,,. .ДҚη5Ж,,W,.=�����(1.16)W(Vmax>>kT).,,.,.W.,H.Sonntage [152Ж.,E. Honig [156Ж, .

.J. Lyklema, [157,158Ж,,.,.. .ДҚ59Ж..,,,.49,,.,,.,.,ДҚθ0-162Ж(«»),,.,.KNO3.,,...,,,«».A. SmithL. Thompson [163]KNO3 ( = 0.0Қr = 0.8/ )–.L. ThompsonD. Pryde [164,165Ж(r = 0.η),,,.,50,J. Cahill [166Ж.,.(r = қ.ηηG. Jeffreyr = Қ.3),R. Ottewill [167Ж.,.,,.,..G. Odriozola [168,169Ж,қ.,қ..,d(lgW)/d(lgC)..,..ДҚ70,171Ж..51,.ДҚ72Ж..,, .

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