Диссертация (1145490), страница 49
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Rodriguez-Mendez Ed.,Academic Press, 2016, P. 149-160.253ПРИЛОЖЕНИЕ 1Табл. 1. Значения коэффициентов селективности для электродов на основе Ptпорфирин-ионофоров (1% по весу) и TДMACl в различных количествах(обозначено как мол% по отношению к содержанию ионофоров), оцененныеметодом БИП. Для вычисления значений logKi/Jpot был использован теоретическийнаклон -59,2 мВ/pI.logKпотI/Х, Х=Мб: CоставBr-NO3-NO2-CO32-Cl-SO42-ClO4-Sal-SCN-F-1: TДМACl, 10%0.260.470.2-2.64-0.85-2.702.080.751.74-1.513:Pt(II)TPPCl2+TДМACl 10%-2.66-1.09-2.43-3.21-3.37-3.00-0.06--0.28-4: Pt(II)TPPCl2+TДМACl 20%-2.52-1.01-2.40-3.00-3.15-2.800.13--0.19-5: Pt(II)TPPCl2+TДМACl 40%-1.04-0.55-1.23-3.40-2.44-3.660.49-0.080.24-2.888: Pt(II)TPP+TДМACl 10%-2.63-2.06-2.55-2.96-2.96-3.100.82-1.110.35-2.619: Pt(II)TPP+ TДМACl 40%-1.49-1.02-1.96-1.91-2.47-2.921.26-0.32-0.05-3.0312: Pt(II)OEP +TДМACl 10%-0.830.190.29-2.60-1.83-2.901.321.311.96-2.0715: Pt(II)OEP +TДМACl 40%-2.23-1.75-2.25-3.80-2.79-3.91-1.27-1.2-3.20Табл.
2. Исходные данные от мультисенсорной системы (величины потенциаловсенсоров в мВ), использованныедля прогнозирования концентрациимикроцистина (MC-LR) методом ПЛС1 регрессии в водопроводной воде,загрязненной фильтратами токсичного штамма M. Aeruginosa, в которыхсодержание токсина определяли методом ЖХ и энзимным колориметрическиманализом. Кодировка образцов: день_месяц_токсичный образец(ТОХ)_добавка вмкл/50мл[MC-LR], мкг/лGCPbGCAgЭнзимныйметод,ЖХметодобразецА1А2А3С1С2GCCu24_03_TOX_0177.3176.3188.765.947.153-201.6286.8mm24_03_TOX_20176.3176.3188.266.446.152-201.6286.81.00E-02m24_03_TOX_30175.8174.8187.766.951.551-205286.32.50E-02m24_03_TOX_50174.3174.8187.267.951.550-207.5285.34.99E-02m24_03_TOX_100172.3173.3186.268.447.149-212283.39.96E-02m24_03_TOX_500165.9173.3184.870.854.547.1-221.4278.80.3452m24_03_TOX_1.5154172.4181.375.362.944.6-236.7267.91.0536m25427_03_TOX_0175.3158179.8m44.637.1-208.5mmm27_03_TOX_20174.8157179.8m45.636.7-210m1.04E-024.50E-0327_03_TOX_30173.8156.5179.3m45.136.2-212m2.60E-021.12E-0227_03_TOX_50172.8156.5179.3m44.135.7-212.5m5.19E-022.25E-0227_03_TOX_100170.9156.5178.8m45.135.7-211m0.10364.48E-0227_03_TOX_500166.9156177.8m46.135.2-216.4m0.3590.155327_03_TOX_1.5160155.5176.8m46.134.7-220.4m1.09580.474131_03_TOX_0123.3149.1189.2m25.842.1-264175.3mm31_03_TOX_20122.8148.6188.7m26.341.1-264.5172.98.40E-032.20E-0331_03_TOX_30122.8148.1188.2m28.240.1-266171.42.10E-025.50E-0331_03_TOX_50122.3147.6187.7m27.839.1-266.9169.44.19E-021.10E-0231_03_TOX_100121.3147.1187.2m28.738.6-267.9167.48.37E-022.20E-0231_03_TOX_500120.8146.6185.7m29.237.1-268.9166.40.28997.62E-0231_03_TOX_1.5119.8146.6183.3m30.735.7-269.9163.90.88510.232603_04_TOX_0122.8157184.825.348.134.2-278.3246.2mm03_04_TOX_20121.8157183.824.35033.2-278.3246.61.28E-021.80E-0303_04_TOX_30121.3156182.822.85232.7-278.8247.13.20E-024.50E-0303_04_TOX_50120.3155.5181.324.853.532.2-279.3248.66.39E-029.00E-0303_04_TOX_100118.9154.5180.321.855.531.2-280.3249.60.12751.79E-0203_04_TOX_500117.4154179.824.35930.2-281.3249.60.44186.21E-0203_04_TOX_1.5110.9154178.329.267.930.2-283.3248.11.34870.189707_04_TOX_0131.2167.4191.747.136.730.2-270.4244.7mm07_04_TOX_20130.7166.4191.245.137.228.7-270.9245.28.00E-03m07_04_TOX_30129.7165.9191.248.536.728.7-272.4243.72.00E-02m07_04_TOX_50129.3164.9190.244.637.727.7-273.9242.23.99E-02m07_04_TOX_100128.3163.9189.747.539.126.7-275.4242.27.97E-02m07_04_TOX_500126.8163.4187.745.145.124.3-277.8241.20.2761m07_04_TOX_1.5124.3163.4183.3555519.8-280.3240.70.8429m10_04_TOX_0105158.5173.45864.934.2-276.8287.8mm10_04_TOX_20104159.5172.95865.433.7-278.3287.38.00E-031.80E-0310_04_TOX_30104157.5172.45866.432.2-278.8286.82.00E-024.50E-0310_04_TOX_50104157171.95865.931.2-280.3285.33.99E-029.00E-0310_04_TOX_100102.5157.5171.458.465.929.7-282.3284.37.97E-021.79E-0210_04_TOX_500102.5155.5170.958.467.927.7-284.8284.30.27616.21E-0225510_04_TOX_1.5101.5159169.958.969.424.8-287.3283.30.84290.189714_04_TOX_096.1127.816365.468.425.3-302.6mmm14_04_TOX_2096.1128.816265.467.923.3-303.1m9.60E-034.20E-0314_04_TOX_3095.6128.3162.564.967.921.3-303.1m2.40E-021.05E-0214_04_TOX_5095.6127.3162.565.468.421.3-304.1m4.79E-022.09E-0214_04_TOX_10095.6127.816265.467.921.8-304.6m9.56E-024.17E-0214_04_TOX_50091.1127.3161.565.967.918.3-305.6m0.33140.144614_04_TOX_1.590.1126.8160.566.468.417.8-307.6m1.01150.441317_04_TOX_093.1153167.969.878.326.7-258101mm17_04_TOX_2093.1152.5167.969.878.825.8-259100.51.00E-021.80E-0317_04_TOX_3093.1151.5167.469.880.325.3-260.51002.50E-024.50E-0317_04_TOX_5092.6152167.469.879.324.3-262.599.54.99E-029.00E-0317_04_TOX_10092.6150.6166.969.879.823.3-26598.19.96E-021.79E-0217_04_TOX_50091.6151.1166.470.379.320.8-268.497.60.34526.21E-0217_04_TOX_1.586.2152164.470.881.217.3-271.993.61.05360.189722_04_TOX_0100.5125.8166.966.478.323.3-283.874.8mm22_04_TOX_20100.5126.3166.466.978.323.3-284.375.88.80E-036.10E-0322_04_TOX_30100.5125.8166.466.479.322.3-284.877.32.20E-021.52E-0222_04_TOX_50100.5124.8166.466.977.822.3-285.877.34.39E-023.04E-0222_04_TOX_100100124.8166.466.977.320.3-286.877.88.76E-026.07E-0222_04_TOX_50099.5125.3165.967.476.818.8-287.775.30.30370.210422_04_TOX_1.599124.8165.967.481.215.4-290.270.30.92720.642324_04_TOX_091.6135.2162.566.970.832.2-274.9136.7mm24_04_TOX_2092.1133.716366.474.331.7-275.4139.2mm24_04_TOX_3091.6133.7162.566.474.330.2-275.9139.7mm24_04_TOX_5091.1134.216266.973.329.7-276.8139.7mm24_04_TOX_10091.1133.7162.566.973.329.2-278.8140.2mm24_04_TOX_50090.6132.716267.473.326.3-279.8139.2mm24_04_TOX_1.589.6131.716267.974.317.8-281.8132.7mm28_04_TOX_0102.5149.1174.468.856.527.7-296.2mmm28_04_TOX_20102.5148.1174.469.35726.7-296.7m6.80E-03m28_04_TOX_30101.5148.1173.969.35827.2-297.7m1.70E-02m28_04_TOX_50101.5147.6171.969.359.526.7-298.1m3.39E-02m28_04_TOX_100101146.6171.969.360.925.8-298.6m6.77E-02m25628_04_TOX_50097.6147.1172.469.862.924.8-299.1m0.2347m28_04_TOX_1.592.6147.1170.970.367.419.8-299.6m0.7165m30_04_TOX_0107.5157.5176.871.35332.2-300.644.1mm30_04_TOX_20107.5157176.870.85331.7-300.642.6mm30_04_TOX_30107.5154.5176.870.853.531.2-302.140.1mm30_04_TOX_50107154176.370.85331.7-301.637.1mm30_04_TOX_100106155176.870.852.530.2-302.636.6mm30_04_TOX_500103152.5175.370.853.529.7-305.133.7mm30_04_TOX_1.594.1153.5172.471.85528.7-30931.2mm05_05_TOX_0100139.7178.347.541.623.3-299.674.3mm05_05_TOX_2099138.7178.34843.122.3-300.173.31.12E-024.00E-0305_05_TOX_3098.5139.2177.847.542.622.8-300.675.82.80E-021.01E-0205_05_TOX_5098.1138.7177.8484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368.434.7-268.42135.1774994.046716_06_TOX_1.5101.5143.1188.270.371.330.7-273.4209.515.8045912.35289106130.7185.7mm26.7-26379.2mm19_06_TOX_025919_06_TOX_20106130.2185.3mm25.8-26679.20.13790.106619_06_TOX_30106130.2185.3mm24.8-267.478.70.34470.266419_06_TOX_50105.5129.8184.3mm25.3-267.478.20.68860.532319_06_TOX_100105.5129.8184.3mm23.8-267.977.31.37451.062519_06_TOX_500105.5129.3183.8mm22.8-271.975.34.7632993.682219_06_TOX_1.5105.5128.3183.3mm21.3-274.971.314.5402011.240223_06_TOX_0177.3176.3188.765.947.153-201.6286.8mm23_06_TOX_20176.3176.3188.266.446.152-201.6286.80.12990.105423_06_TOX_30175.8174.8187.766.951.551-205286.30.32470.263223_06_TOX_50174.3174.8187.267.951.550-207.5285.30.64870.525923_06_TOX_100172.3173.3186.268.447.149-212283.31.29481.049823_06_TOX_500165.9173.3184.870.854.547.1-221.4278.84.4871983.63809923_06_TOX_1.5154172.4181.375.362.944.6-236.7267.913.697311.10540Табл.
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